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The last voyage of the Karluk, flagship of the Canadian Arctic Expedition of 1913–16, ended with the loss of the ship in the Arctic seas, and the subsequent deaths of nearly half her complement of 25.

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Here, we present a computational structure-based redesign of the 65-kDa phenylalanine adenylation domain of the nonribosomal peptide synthetase (NRPS) enzyme gramicidin S synthetase A (GrsA-PheA) for a set of noncognate substrates.